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A visible-light-mediated hydrotrifluoromethylation of unactivated alkenes that uses the Umemoto reagent as the CF(3) source and MeOH as the reductant is disclosed. This effective transformation operates at room temperature in the presence of 5 mol % Ru(bpy)(3)Cl(2); the process is characterized by its operational simplicity and functional group tolerance.

Original publication

DOI

10.1021/ja401022x

Type

Journal article

Journal

J Am Chem Soc

Publication Date

20/02/2013

Volume

135

Pages

2505 - 2508

Keywords

Alkenes, Catalysis, Fluorine, Methylation, Molecular Structure